Organic and Elemental Carbon in Atmospheric Fine Particulate Matter in an Animal Agriculture Intensive Area in North Carolina: Estimation of Secondary Organic Carbon ConcentrationsReport as inadecuate




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Carbonaceous components contribute significant fraction of fine particulate matter PM2.5. Study of organic carbon OC and elemental carbon EC in PM2.5 may lead to better understanding of secondary organic carbon SOC formation. This year-long December 2008 to December 2009 field study was conducted in an animal agriculture intensive area in North Carolina of United States. Samples of PM2.5 were collected from five stations located in an egg production facility and its vicinities. Concentrations of OC-EC and thermograms were obtained using a thermal-optical carbon analyzer. Average levels of OC in the egg production house and at ambient stations were 42.7 μg-m3 and 3.26 - 3.47 μg-m3, respectively. Average levels of EC in the house and at ambient stations were 1.14 μg-m3 and 0.36 - 0.42 μg-m3, respectively. The OC to total carbon TC ratios at ambient stations exceeded 0.67, indicating a significant fraction of SOC presented in PM2.5. Principal factor analysis results suggested that possible major source of in-house PM2.5 was from poultry feed and possible major sources of ambient PM2.5 was from contributions of secondary inorganic and organic PM. Using the OC-EC primary ratio analysis method, ambient stations SOC fractions ranged from 68% to 87%. These findings suggested that SOC could appreciably contribute to total PM2.5 mass concentrations in this agriculture intensive area.

KEYWORDS

Secondary Organic Carbon SOC; Organic Carbon OC; Elemental Carbon EC; PM2.5; Agriculture Area

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Q. Li, L. Wang-Li, R. Jayanty and S. Shah -Organic and Elemental Carbon in Atmospheric Fine Particulate Matter in an Animal Agriculture Intensive Area in North Carolina: Estimation of Secondary Organic Carbon Concentrations,- Open Journal of Air Pollution, Vol. 2 No. 1, 2013, pp. 7-18. doi: 10.4236-ojap.2013.21002.





Author: Qian-Feng Li, Lingjuan Wang-Li, R. K. M. Jayanty, Sanjay B. Shah

Source: http://www.scirp.org/



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